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Match Recap: Men's Tennis | 3/16/2025 6:31:00 PM | Evan Snyder / MTSU Athletic Communications
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The 5-year old Freiherr Peter and the 6-year old Visser's Hit Valeria VEC became the winners of the rather small Bundeschampionate qualification classes held at the dressage show in Vöhl on Sunday 30 April 2023
Seven 5-year olds competed in the L-level dressage horse test but no horses obtained a high enough score to clinch a ticket to Warendorf
The winner of the class was Mareike Mimberg-Hess aboard Peter Kremer's home bred Westfalian gelding Freiherr Peter (by Furstenball x Sandro Hit)
The pair topped the board with a total of 7.60
aboard Bianka Schulte-Krist's Westfalian gelding Di Nozzo (by Dantano x L'Espoir)
In the 6-year old division five pairs battled it out and one combination scored enough to make it to Warendorf: the winner of the class
Nicole Grosch aced the M-level dressage horse test aboard Sven Hecht's Oldenburg mare Visser's Hit Valeria VEC (by Vitalis x Diamond Hit)
They received a winning 8.40 points from judges Ute Kombächer
Two pairs tied in second place on a score of 7.50 pounts: Björn Steigauf on Jillian Wyrobnik's DSP stallion Floriano (by Floriscount x Alabster) and Hanna Rüther aboard Stephanie Schnettler's Oldenburg gelding Bugatti Gold (by Best of Gold x Sandro Hit)
Stalls for Rent at Durondeau Dressage in Peer, Belgium
Exceptionally Well Located Equestrian Facility in Wellington, Florida
Well-built Equestrian Estate With Multiple Business Opportunities in Sweden
Stable Units for Rent at Lotje Schoots' Equestrian Center in Houten (NED)
For Rent: Several Apartments and Stable Wing at High-End Equestrian Facility
Stable Wing Available at Reiterhof Wensing on Dutch/German border
Real Estate: Well-Appointed Country House with Extensive Equestrian Facility in the U.K.
Rémi Blot
A community bulletin board for Western Pierce County
Susanne Bacon · March 21
My first encounters with Americans as an adult usually started with them trying out the few German words they knew on me
and to run into them when going out was a given
was that one of their first German terms they used on me often was “Jawohl”(pronounce: yah-‘vohl) or “Jawoll” (pronounce: yah-‘voll)
why did they reply in a way as if I were outranking them in a military hierarchy
The answer is simple – watch any older movie about Third Reich Germany (I don’t think there are any about the German Empire)
and at one point or another you’ll find the caricature of a German soldier saluting his commander with “Jawoll” or “Jawohl”
I never thought this was a Germanism in the English language
I rather always thought it a bad JOKE because the Third Reich and its militarism AREN’T a joke to Germans
Being answered “Jawohl” or “Jawoll” feels a little like being needled about a nation’s past that is more than shameful
I’m not sure whether the German military still uses this word as a reply to the order of another military member
It is more of a passive term in the civilians’ vocabulary
“nein” can also express an implicit prohibition or an exclamation of surprise whereas “ja” can be used as cheering somebody on
There is one variant of the German “ja” that expresses a sigh – it’s “jaja”
It expresses either nostalgia when muttered more to oneself
Or boredom and irritation when replied to somebody else’s utterance
Which is why I end this article here and now before you yawn at me
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I look forward to reading your posts in the Suburban Times
You present a rich knowledge of your German ancestry in the culture
and stories and find humor in the way you do that
I know I have met you at some occasion(s) in Steilacoom
You start off my daily network activities in an uplifting way
Copyright © 2025 · The Suburban Times · Log in
“How do you feel?” Her wind-chime words are meant for the many men who died in this bedroom almost 150 years ago, in pain.
Dion, deeper-pitched, speaks with authority. “If you want to talk to us, go to that light.” The pinprick-sized glow, red like fresh blood, comes from a plastic box on the 19th-century oak floor. It’s a combination motion sensor and electromagnetic field (EMF) detector.
We sit in a circle around the machine and wait for it to screech, which would indicate motion, possibly of the paranormal sort. Or perhaps a surge in the surrounding electromagnetic field will make the needle thwap across the screen like a smack in the face. This may represent a ghost (or, I remind myself, a m…
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Illustrations by Julia Vohl\u201CIs anybody here?\u201D Silence
\u201CWe\u2019d love to talk with you.\u201D Silence
\u201CCan you make a sound for us?\u201D Diane\u2019s voice creeps upward through the blackness with a tinge of desperation
\u201CHow do you feel?\u201D Her wind-chime words are meant for the many men who died in this bedroom almost 150 years ago
go to that light.\u201D The pinprick-sized glow
comes from a plastic box on the 19th-century oak floor
It\u2019s a combination motion sensor and electromagnetic field (EMF) detector
We sit in a circle around the machine and wait for it to screech
Or perhaps a surge in the surrounding electromagnetic field will make the needle thwap across the screen like a smack in the face
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Robotic microscopes revolutionize biological research by automating cell tracking
and enabling longitudinal studies on diseases
Consumer drones are reshaping how we think about privacy
blurring the lines between public airspace and personal space
Feedback systems are crucial for robotic autonomy
enabling real-time adaptation and decision-making for safe and efficient operation in various environments
Discover Cavitar’s welding cameras that can be used in a variety of situations to offer high-quality visualization of the welding processes
MTI’s 1510A portable signal generator and calibrator is ideal for testing the integrity of sensor signal conditioning electronics
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Photo by: Ken ShepherdMen's Tennis Defeats Tulane
6-11/29/2025 8:17:00 PM | Men's Tennis
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NADH oxidation is coupled to ion translocation across the membrane to build up an electrochemical gradient
the sodium-pumping NADH:quinone oxidoreductase (Na+-NQR) generates a sodium gradient by a so far unknown mechanism
Here we show that ion pumping in Na+-NQR is driven by large conformational changes coupling electron transfer to ion translocation
We have determined a series of cryo-EM and X-ray structures of the Na+-NQR that represent snapshots of the catalytic cycle
and F of Na+-NQR harbor a unique set of cofactors that shuttle the electrons from NADH twice across the membrane to quinone
The redox state of a unique intramembranous [2Fe-2S] cluster orchestrates the movements of subunit NqrC
We propose that this switching movement controls the release of Na+ from a binding site localized in subunit NqrB
and the positions of side chains and the cofactor riboflavin were not unambiguously resolved
The high-resolution cryo-EM structures reported here reveal the exact localization and nature of all cofactors
including a [2Fe-2S] cluster in subunits NqrD and NqrE
Overall structure of Na+-NQR in complex with NADH and ubiquinone-2
Structure of Na+-NQR determined by X-ray crystallography
Both structures differ in the position of the periplasmic hydrophilic domain of NqrC
Structural overlay of the cryo-EM (red) and X-ray (gray) structures of NqrF bound to NADH and UQ-2
NqrD (magenta) and NqrE (cyan) are shown as surface
the FNR-like domain of NqrF is shifted sideways
and the ferredoxin (Fdxn)-like domain is rotated towards the membrane subunits in the cryo-EM structure
Edge-to-edge distances of redox cofactors in Na+-NQR determined by cryo-EM
Edge-to-edge distances of redox cofactors in Na+-NQR determined by X-ray crystallography
Gray bars indicate the location of the membrane
Close-up view of subunits NqrD-E coordinating a [2Fe-2S] cluster
with cysteines originating from both subunits
Localization of the [2Fe-2S] clusters in cytoplasmic NqrF and in membrane subunits NqrD-E
The blue circle indicates the [2Fe-2S]NqrF cluster; the red circle indicates the [2Fe-2S]NqrD-E cluster
CD spectra of wild-type (WT) Na+-NQR; NqrF-C70A
which is devoid of [2Fe-2S]NqrF; and NqrD-C29A
the [2Fe-2S]NqrD-E cluster (red trace) in NqrF-C70A
and the [2Fe-2S]NqrF cluster (blue trace) in NqrD-C29A are shown
k3-weighted EXAFS and Fourier transform spectra of cluster [2Fe-2S]NqrD-E (red) in NqrF-C70A
and cluster [2Fe-2S]NqrF (blue) in NqrD-C29A
57Fe Mössbauer spectrum of the [2Fe-2S]NqrD-E cluster in NqrF-C70A
10 K X-band EPR spectrum of Na+-NQR variant NqrF-C70A showing [2Fe-2S]NqrD-E cluster
simulated with two components: a [2Fe-2S] cluster (orange; g|| = 2.02
line width = 50 G) and a radical signal (purple; giso = 2.01
cholerae expressing WT Na+-NQR (black) or Na+-NQR variants containing cluster [2Fe-2S]NqrD-E (red) in variant NqrF-C70A or cluster [2Fe-2S]NqrF (blue) in variant NqrD-C29A
Source data
Structural alignment of Na+-NQR in two states
highlighting the two conformations of NqrC trapped in cryo-EM and X-ray structures
The membrane plane is indicated by gray bars
The movement of NqrC corresponds to a 26-degree rotation of the hydrophilic domain
green spheres) binds to the rim of NqrB with the head group close to the cytoplasmic aspect of the membrane
Interactions of UQ-1 (b) and UQ-2 (c) with NqrB
The isoprenoid and the methyl group are in hydrophobic contact with residues F159
whereas the O4 can form a hydrogen bond to a backbone carbonyl of N156
Replacement of G141 with any other amino acid residue would sterically block the interaction of quinones with NqrB
at the N terminus of NqrB close upon UQ binding and contribute to the mainly hydrophobic interaction of UQ-1 or UQ-2 with NqrB
The methoxy groups of the quinone head group are in hydrophobic contact with the side chains of L26
These interactions are critical and stabilize the bound cofactor in this position in an induced-fit binding mode
Structural alignment of Na+-NQR in complex with either UQ-1 or with HQNO
The binding sites for both molecules overlap
but head groups and tails localize in different regions of the binding site
The quinolone head group of HQNO interacts with the side chain of F160 and L33
The alkyl chain of HQNO covers the space of the head group of quinones and follows the course of the isoprenoid tail
HQNO recruits the N-terminal amphiphilic helices to form a high-affinity binding site
cholerae is replaced by a phenylalanine in NqrB of P
aeruginosa that predicts that HQNO binding is indeed hampered by the bulky side chain of phenylalanine
This strongly suggests that the different conformation of NqrC in the X-ray structure is due to the crystallization of Na+-NQR
The conformational change is not due to pH or ionic strength of the crystallization conditions
because these are similar to the buffer conditions used for the cryo-EM samples
We concluded that the packing of the Na+-NQR in the crystal provides enough energy to stabilize NqrC in its position at NqrD-E
the subunit arrangement observed in the X-ray structure is largely stabilized by the packing of the molecules in the crystal
NqrC interacts in the crystal with two neighboring Na+-NQR molecules
forming three salt bridges and several hydrogen bonds
thus stabilizing a conformation that represents a certain state of the catalytic cycle
Because this state is not observed at thermodynamic equilibrium
it is most likely a transient or metastable state that is trapped by the crystal packing
The close proximity of FMNNqrC to [2Fe-2S]NqrD-E
suggests that it represents a snapshot of transmembrane electron transfer
as shown by experiments treating the protein in the crystals with the inhibitor DQA
incubation of the crystals with the inhibitor triggered a large conformational change of NqrC
NqrC does not reach the final relaxed position at NqrB that was observed in the cryo-EM structures
and some residual crystal contacts capture Na+-NQR in a transient state
we can distinguish three conformations of Na+-NQR that reflect different states: (1) the relaxed state
as observed in the cryo-EM structures; (2) a short-lived transmembrane electron-transfer state that is shown in the X-ray structure of Na+-NQR; and (3) an intermediate state between these two states
obtained after treatment of the crystals with DQA
A systematic analysis of the structures revealed that the states differ not just in the position of NqrC, but also in the conformation of NqrD-E and in the position and interhelical angles of the transmembrane helices of NqrC and NqrF (Extended Data Fig. 8)
showing that the various movements of the different subunits are tightly interconnected
Helix-III and the half-helix-IV of NqrE tilt and move by 6–10 Å
NqrD and NqrE are related by an inverted topology and form a compact dimer
any conformational changes in one of these subunits will affect the other
NqrD and NqrE are tightly coupled to each other: conformational changes of helix-III and half-helix-IV of NqrE are linked to conformational changes of helix-III and half-helix-IV of NqrD in the opposite direction
This additional negative charge might attract the positive dipole of one half-helix and repulse the negative dipole of the second half-helix
promoting the reorientation of the helices
Two ion-binding sites were identified in NqrB
Both sites are located close to the periplasmic aspect of NqrB
and the Na+ ion is coordinated by three backbone carbonyl oxygen atoms and two water molecules
with a coordination sphere of four backbone carbonyl oxygens and one water molecule
A Na+-translocation pathway through NqrB is predicted
The translocation pathway is constricted close to residues F338 and F342
The results corroborate that F338 and F342 in NqrB are critically involved in Na+ translocation
given suitable distances between the redox cofactors
electron transfer is several orders of magnitudes faster than ion translocation
If all six redox cofactors would reside in short distance from each other suited for fast electron transfer
the ion-translocation process would be too slow to be connected to several electron-transfer steps; that is
the energy of the different redox steps would deflagrate
To couple electron transfer to the Na+-pumping process
the system has to decelerate electron transfer at certain steps to allow ion translocation to proceed
Such slow phases are intimately linked to states of Na+-NQR
in which we observe large distances between the redox centers; that is
the distance between the redox centers has to increase
conformational changes will again move redox centers within the electron-transfer distance for fast electron transfer
The catalytic cycle starts with NADH becoming oxidized at NqrF
Electrons are transferred to the flexibly tethered ferredoxin-like domain of NqrF
A Na+ is bound in NqrB close to the periplasmic half-channel
but the release of the ion is blocked by NqrC
NqrD-E adopt a conformation that allows access of the intramembranous [2Fe-2S]NqrD-E cluster from the cytoplasmic side
whereas access for NqrC at the periplasmic side is blocked
The ferredoxin-like domain of NqrF can reach the [2Fe-2S]NqrD-E cluster and transfers an electron
This electron transfer prepares for binding of a Na+ to the cytoplasmic half-channel in NqrB
The reduction of [2Fe-2S]NqrD-E triggers a conformational switch in subunits NqrD-E
now obstructing the access of [2Fe-2S]NqrD-E at the cytoplasmic side but facilitating access of NqrC at the periplasmic side
NqrC rotates from its position at NqrB towards NqrD-E and triggers the release of the Na+ bound at the periplasmic side in proximity of FMNNqrB
The conformational change of NqrC locates FMNNqrC close to [2Fe-2S]NqrD-E resulting in fast electron transfer to the flavin
Oxidation of the [2Fe-2S]NqrD-E cluster will switch NqrD-E back to its previous conformation
the electron is transferred rapidly to FMNNqrB
It is proposed that the reduced FMNNqrB triggers a transient opening between both half-channels in NqrB
enabling translocation of the Na+ to the periplasmic half-channel
NqrB is reoxidized by electron transfer to riboflavinNqrB and subsequently to ubiquinone
Our results provide a detailed model of dynamic conformational coupling of electron transfer to Na+ translocation in Na+-NQR of the human pathogen V
This exemplifies how redox energy is converted into a chemiosmotic gradient by a respiratory complex
Na+-NQR is crucial for energy conservation in a plethora of Gram-negative pathogenic bacteria
including multidrug-resistant species like Klebsiella spp
The structural information on HQNO binding forms an excellent basis for the development of new antibiotics
hexahistidine-tagged Na+-NQR was expressed in V
Membranes were isolated and solubilized with n-dodecyl-β-d-maltoside (DDM; Glycon)
Na+-NQR was purified via Ni-Sepharose Fast Flow (Cytiva) utilizing the N-terminal hexahistidine tag fused to subunit NqrA
Purified Na+-NQR was dialyzed against 50 mM sodium phosphate
Na+-NQR was concentrated by ultrafiltration (Amicon
100-kDa cut-off) and further purified by size-exclusion chromatography using a Superdex 200 (16/60) column (GE Healthcare) equilibrated in 50 mM HEPES-NaOH
the hexahistidine tag was removed from NqrA by proteolysis with HRV-3C protease carrying a hexahistidine tag on ice prior to gel filtration
The digest was supplemented with 0.25 μM phenylmethylsulfonyl fluoride and passed again over Ni-Sepharose Fast Flow (Cytiva) in order to remove undigested protein
Na+-NQR (wild-type or variants) was purified as described above
Na+-NQR in buffer (50 mM potassium phosphate
5 % glycerol) was flash-frozen in liquid N2 and stored at −80 °C until use
the Na+-NQR complex was prepared at a concentration of 1 mg ml–1 in 10 mM HEPES pH 8.0
Fifty-microliter aliquots (50 µg protein) were used for the experiments
Na+-NQR was cross-linked in the absence and presence of the inhibitor DQA
DQA was added from a 50 mM stock in DMSO to a final concentration of 0.5 mM
Samples were incubated for 45 min at room temperature before cross-linking
Cross-linking was performed using a mixture of isotopically light (d0) and heavy (d12) di(succinimidyl)suberate (DSS-d0/d12
DSS was added to a final concentration of 1 mM from a 25 mM stock solution prepared in DMF
and samples were incubated for 45 min at 25 °C
ammonium bicarbonate was added to a final concentration of 50 mM from a 1 M stock solution prepared in water
and samples were incubated for another 20 min
For reduction and alkylation of cysteine residues
tris(2-carboxyethyl)phosphine (50 mM in water) was added to a final concentration of 5 mM
and the sample was incubated for 30 min at 37 °C
iodoacetamide (100 mM in water) was added to a final concentration of 10 mM
and samples were incubated at room temperature for 30 min in the dark
This step was followed by the addition of 0.5 µg endoproteinase Lys-C (Wako
and digestion was allowed to proceed for 2.5 h at 37 °C
Sample solutions were diluted to a final volume of 400 µl with 50 mM ammonium bicarbonate (which diluted DDM below the CMC)
Three fractions corresponding to the predominant elution range of cross-linked peptides were collected separately for mass spectrometry and were evaporated to dryness
Dried SEC fractions were dissolved in 20 µl of water/acetonitrile/formic acid (95/5/0.1
and 4 µl was analyzed in duplicate on a liquid chromatography–mass spectrometry system consisting of an Easy nLC-1200 HPLC system and an Orbitrap Fusion Lumos mass spectrometer (both Thermo Fisher Scientific)
Peptides were separated on an Acclaim PepMap RSLC C18 column (25 cm × 75 µm
Thermo Fisher Scientific) at a flow rate of 300 nl min–1 and with a gradient of 89% mobile phase A/11% mobile phase B to 60% A/40% B in 60 min
where A is water/acetonitrile/formic acid (98/2/0.15
vol/vol/vol) and B is acetonitrile/water/formic acid (80/20/0.15
Peptides were sequenced in the data-dependent acquisition mode with precursor ion scans acquired in the orbitrap analyzer at a resolution of 120,000
The most abundant precursors with a charge state of +3 or higher were selected for sequencing by collision-induced dissociation in the linear ion trap at a normalized collision energy of 35%
and fragment ions were detected in the linear ion trap at rapid speed
The cycle time for sequencing was set to 3 s
and dynamic exclusion was enabled after one sequencing event for 30 s
DSS specificity was set to only lysine residues
Mass error tolerances for the xQuest search were set to ± 15 ppm at the MS1 level and to 0.2 Da and 0.3 Da (for common and xlink ion types
Relative changes in the abundance of cross-linked peptide pairs are given as +DQA/–DQA ratios
Ratios were median-normalized and averaged over charge states and were determined for light and heavy DSS products
The amino acid sequence of NqrF from V. cholerae (residues 129–408) representing the FNR-like NADH-oxidizing domain2 was obtained from Uniprot (ID: A5F5Y4)
An N-terminal 6×His-tag and a subsequent HRV-3C cleavage site were added
and codons were optimized for expression in Escherichia coli
Genes coding for NqrF129-408 and NqrF129-408-F406A were synthesized by GeneArt (Thermo Fisher Scientific) and cloned into vector pET15b via flanking 5′ NcoI and 3′ BamHI
replacing the 6×His-tag and thrombin-cleavage site of pET15b
coli Tuner (DE3) strain was transformed with plasmid pFNF53 or pFNF406A
Cells were grown in DYT medium containing 100 µg ml−1 ampicillin at 37 °C
Expression of the FAD domain was induced with 1 mM IPTG at an OD600 of 0.9
Cells were collected after 5 h at 30 °C and washed in 10 mM Tris-HCl
Cells were broken by one passage through an Emulsiflex C-3 cell disruptor (Avestin) at approximately 20 kpsi in the presence of 1 mM DTT and protease inhibitors (complete EDTA-free
Cell debris was removed by centrifugation at 20,000g for 20 min
After ultracentrifugation of the cellular extract at 150,000g (Beckman Type 70Ti)
the supernatant was filtrated and loaded onto a Ni Sepharose HP column (5 ml bed volume
Cytiva) equilibrated with buffer A (20 mM Tris-HCl
The column was washed with 5 volumes of buffer A containing 30 mM imidazole
and histidine-tagged protein was eluted with 400 mM imidazole in buffer A
Peak fractions were combined and diluted at least 1:10 in 50 mM HEPES-NaOH
The histidine tag was cleaved off by incubation for 15 h at 4 °C with PreScission protease
By loading the digest onto the Ni+ column and washing with 50 mM HEPES-NaOH
FAD domain devoid of the histidine tag was obtained
The protein was loaded onto a SourceQ column (10 ml bed volume
Cytiva) equilibrated with 50 mM HEPES-NaOH
and was eluted with a linear gradient from 0 to 0.4 M NaCl
and proteins were frozen in liquid nitrogen
Point mutations were introduced into plasmid pNqr1 by a single PCR reaction (KAPAHiFi PCR Kit
Peqlab) with the corresponding forward and reverse primers
Mutated codons that introduce the altered amino acid residues in the Nqr subunits are underlined
Plasmid pNF-C70A codes for Na+-NQR carrying the p.C70A substitution in NqrF
5′-GTATTCGTATCTTCAGCTGCGGGTGGTGGTGGTTCATGTGG-3′ and 5′-CCACATGAACCACCACCACCCGCAGCTGAAGATACG-3′
Plasmid pND-C29A codes for Na+-NQR carrying the p.C29A substitution in NqrD
The forward and reverse primers were 5′-TTCTGGGTGTGGCGCTGCACTGGC-3′ and 5′-CCAGTGCAGACGCCACACCCAGAAC-3′
Plasmid pNDE-C29A-C120A codes for Na+-NQR carrying the p.C29A substitution in NqrD and the p.C120A substitution in NqrE
Substitution p.C29A was inserted with the same forward and reverse primers like in pND-C29A
the forward and reverse primers were 5′-GATCACAGTAAACGCGGCGATCTTCGG-3′ and 5′-GAAGATCGCCGCGTTTACTGTGATCAGC-3′
Plasmid pNE-C120S codes for Na+-NQR carrying the p.C120S substitution in NqrE
The forward and reverse primers were 5′-GATCACAGTAAACTCAGCGATCTTCGGTGG-3′ and 5′-ACCGAAGATCGCTGAGTTTACTGTGATCAGC-3′
The enrichment of 57Fe in Na+-NQR was at least 70%
as confirmed by inductively coupled mass spectroscopy
A second-order polynomial was fit to the pre-edge region and subtracted throughout the entire EXAFS spectrum
A three-region cubic spline (with the AUTOBK function within Athena) was used to model the background function to a minimum of k = 13.5 Å−1 for all spectra
Fourier transforms were performed over a windowed k range of 2.0–13.0 Å−1 and all FT spectra are presented without a phase-shift correction
Spectra were collected in a dual-mode X-band resonator operated in perpendicular-mode (TE102)
Magnetic circular dichroism spectra of Na+-NQR (10–20 mg ml−1) were recorded on a Jasco J-715 magnetic circular dichroism (MCD) spectrometer equipped with a permanent 1.6 T magnet
Measurements were performed at room temperature using a 2 mm quartz cuvette at a speed of 100 nm min−1
A magnetic field was applied and –MCD and +MCD spectra were recorded
These spectra were used to calculate CD spectra using the formula: +MCD + –MCD = 2 CD
UV-visible spectra were recorded on a Lambda 12 UV/VIS spectrophotometer (Perkin Elmer) at 19 °C
Absorbance of Na+-NQR (50–100 µM) after gel filtration in 10 mM HEPES pH 8.0
and 0.05% DDM was measured in a 1 mm quartz cuvette
Point mutations were introduced into plasmid pNqr1 by a single PCR reaction (KAPAHiFiTM PCR Kit
from Peqlab) with the corresponding forward and reverse primers
Plasmid pNF-D346A codes for Na+-NQR carrying the p.D346A substitution in NqrB
The forward and reverse primers were 5′-GTTCTTCATGGCGACTGCGCCAGTTTCTGCGTC-3′ and 5′-GAAGGACGCAGAAACTGGCGCAGTCGCCATGAAG-3′
Plasmid pNB_F342A codes for Na+-NQR carrying the p.F342A substitution in NqrB
The forward and reverse primers were 5′-CGCATTCGGTATGTTCGCTATGGCGACTGACCC-3′ and 5′-GAAACTGGGTCAGTCGCCATAGCGAACATACCG-3′
Bandelin) in a 1.5-mL reaction tube on ice
The tip was placed 1 cm below the surface of the proteoliposome suspension
with cooling times of 60 s between the pulses
To decrease the detergent concentration below the critical micellar concentration (CMC)
the suspension was diluted with a 50-fold volume of reconstitution buffer using a burette (30 drops min−1)
the pellet containing the proteoliposomes was suspended in 1 ml reconstitution buffer per 1 mg Na+-NQR
corresponding to 2 ml reconstitution buffer per 40 mg l-α-phosphatidylcholine
proteoliposomes (0.16 mg Na+-NQR in 3.2 mg lipids) were mixed with 6 µM oxonol VI
which was identical to the reconstitution buffer
the reaction was started by the addition of 0.2 mM NADH (dipotassium salt)
and voltage formation was followed at 25 °C under stirring
Typical traces from three replicates are presented
Vectors were created to express Na+-NQR variants carrying cysteine substitutions
Further information on research design is available in the Nature Portfolio Reporting Summary linked to this article
regulation and function of the mitochondrial respiratory chain
cholerae Na+-pumping NADH:quinone oxidoreductase
The Na+/e− stoichiometry of the Na+-motive NADH: quinone oxidoreductase in Vibrio alginolyticus
Cryo-EM structures of Na+-pumping NADH-ubiquinone oxidoreductase from Vibrio cholerae
Identification and evolution of dual-topology membrane proteins
Analysis of Pseudomonas aeruginosa 4-hydroxy-2-alkylquinolines (HAQs) reveals a role for 4-hydroxy-2-heptylquinoline in cell-to-cell communication
Characterization of the Pseudomonas aeruginosa NQR complex
a bacterial proton pump with roles in autopoisoning resistance
Incorporating protein environments in density functional theory: a self-consistent reaction field calculation of redox potentials of [2Fe2S] clusters in ferredoxin and phthalate dioxygenase reductase
Acid residues in the transmembrane helices of the Na+-pumping NADH:quinone oxidoreductase from Vibrio cholerae involved in sodium translocation
Structure and permeation mechanism of a mammalian urea transporter
Mechanism of ammonia transport by Amt/MEP/Rh: structure of AmtB at 1.35 Å
Crystal structure of the archaeal ammonium transporter Amt-1 from Archaeoglobus fulgidus
Metal–ligand geometry relevant to proteins and in proteins: sodium and potassium
Validation of metal-binding sites in macromolecular structures with the CheckMyMetal web server
The role and specificity of the catalytic and regulatory cation-binding sites of the Na+-pumping NADH:quinone oxidoreductase from Vibrio cholerae
Strong pH dependence of coupling efficiency of the Na+-translocating NADH:quinone oxidoreductase (Na+-NQR) of Vibrio cholerae
HOLE: a program for the analysis of the pore dimensions of ion channel structural models
Transport and pharmacological properties of nine different human Na,K-ATPase isozymes
Mechanism of the rate-determining step of the Na +,K + -ATPase pump cycle
Role of the Na+-translocating NADH:quinone oxidoreductase in voltage generation and Na+ extrusion in Vibrio cholerae
Purification and structural characterization of the Na+-translocating ferredoxin: NAD+ reductase (Rnf) complex of Clostridium tetanomorphum
Oxidant-induced formation of a neutral flavosemiquinone in the Na+-translocating NADH:quinone oxidoreductase (Na+-NQR) from Vibrio cholerae
Purification and characterization of the recombinant Na+-translocating NADH:quinone oxidoreductase from Vibrio cholerae
Crystallization of the Na+-translocating NADH:quinone oxidoreductase from Vibrio cholerae
DA+ data acquisition and analysis software at the Swiss Light Source macromolecular crystallography beamlines
MxCuBE: a synchrotron beamline control environment customized for macromolecular crystallography experiments
ANODE: anomalous and heavy-atom density calculation
REFMAC 5 for the refinement of macromolecular crystal structures
Automatic multiple-zone rigid-body refinement with a large convergence radius
AceDRG: a stereochemical description generator for ligands
General atomic and molecular electronic structure system
Real-space refinement in PHENIX for cryo-EM and crystallography
Electronic ligand builder and optimization workbench (eLBOW): a tool for ligand coordinate and restraint generation
New tools for automated cryo-EM single-particle analysis in RELION-4.0
RELION: implementation of a Bayesian approach to cryo-EM structure determination
MotionCor2: anisotropic correction of beam-induced motion for improved cryo-electron microscopy
CTFFIND4: fast and accurate defocus estimation from electron micrographs
Positive-unlabeled convolutional neural networks for particle picking in cryo-electron micrographs
Improvement of cryo-EM maps by density modification
Highly accurate protein structure prediction with AlphaFold
AlphaFold Protein Structure Database: massively expanding the structural coverage of protein-sequence space with high-accuracy models
Model-based local density sharpening of cryo-EM maps
Valence screening of water in protein crystals reveals potential Na+ binding sites
CheckMyMetal: a macromolecular metal-binding validation tool
Lysine-specific chemical cross-linking of protein complexes and identification of cross-linking sites using LC-MS/MS and the xQuest/xProphet software pipeline
False discovery rate estimation for cross-linked peptides identified by mass spectrometry
A cross-platform toolkit for mass spectrometry and proteomics
Identification of cross-linked peptides from large sequence databases
Empirical scoring functions for advanced protein−ligand docking with PLANTS
An ant colony optimization approach to flexible protein–ligand docking
Lessons learned in empirical scoring with smina from the CSAR 2011 benchmarking exercise
new empirical halogen bond scoring function
pK(a) based protonation states and microspecies for protein-ligand docking
Growth yield increase linked to caffeate reduction in Acetobacterium woodii
Semi-micro methods for analysis of labile sulfide and of labile sulfide plus sulfane sulfur in unusually stable iron-sulfur proteins
Design and characterization of phosphine iron hydrides: toward hydrogen-producing catalysts
A function minimization computer package (MFIT) for nonlinear parameter estimation providing readily accessible maximum likelihood estimates
The five-analyzer point-to-point scanning crystal spectrometer at ESRF ID26
HEPHAESTUS: data analysis for X-ray absorption spectroscopy using IFEFFIT
Histidine-gated proton-coupled electron transfer to the Cu A site of nitrous oxide reductase
Reconstitution of sodium transport from purified oxaloacetate decarboxylase and phospholipid vesicles
Comparison of liposomes formed by sonication and extrusion: rotational and translational diffusion of an embedded chromophore
Quinone reduction by the Na+-translocating NADH dehydrogenase promotes extracellular superoxide production in Vibrio cholerae
The Na+-translocating NADH:quinone oxidoreductase enhances oxidative stress in the cytoplasm of Vibrio cholerae
The single NqrB and NqrC subunits in the Na+-translocating NADH: quinone oxidoreductase (Na+-NQR) from Vibrio cholerae each carry one covalently attached FMN
The PRIDE database resources in 2022: a hub for mass spectrometry-based proteomics evidences
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This work was supported by grant 311211092 from the Deutsche Forschungsgemeinschaft (G.F
and by fellowships from the Carl-Zeiss-Foundation (B.C.)
the Landesgraduiertenförderung Baden-Württemberg (V.M.)
Synchrotron data were collected under proposal MX-346 at beamline P14 operated by EMBL Hamburg at the PETRA III storage ring (DESY
Germany) and at beamlines X06SA and X06DA at Swiss Light Source of the Paul Scherrer Institute (Villigen
We thank the Central Electron Microscopy Facility of the Max Planck Institute of Biophysics for excellent support
Yildiz and the Max Planck Computing and Data Facility for maintaining the computational infrastructure for cryo-EM
the staff at beamlines X06SA and X06DA at Swiss Light Source
The HERFD-XAS experiments were performed on beamline ID-26 at the European Synchrotron Radiation Facility (ESRF)
Amidani at ESRF for assistance at beamline ID-26
for access to laboratory infrastructure and instrumentation
Open access funding provided by Universität Hohenheim
Jann-Louis Hau, Valentin Muras, Marco S
Casutt, Georg Vohl, Björn Claußen, Wojtek Steffen, Julia Steuber & Günter Fritz
Max Planck Institute for Chemical Energy Conversion
performed crystallization and data collection
performed XAS experiments and analyzed data
performed EPR and Mössbauer experiments and analyzed data
prepared cryo-EM samples and performed data collection
processed the cryo-EM data and performed model building and refinement
The authors declare no competing interests
: Nature Structural & Molecular Biology thanks Leonid Sazanov and the other, anonymous, reviewer(s) for their contribution to the peer review of this work. Primary Handling Editors: Carolina Perdigoto and Katarzyna Ciazynska, in collaboration with the Nature Structural & Molecular Biology team. Peer reviewer reports are available
Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations
Representative micrograph of Na+-NQR with UQ-1
Gold-standard Fourier Shell Correlation curves and maps colored by local resolution (color scale in Å)
Source data
Several lipids and DDM molecules were well defined by the cryo-EM density
The bound lipids and detergent molecules define the extent of membrane indicated here by grey lines
DDM detergent molecules are depicted in grey
Complex of NADH with NqrF in Na+-NQR cryo-EM structure
The C4N of the nicotinamide group of NADH carrying the 2 e− is at a distance of 3.3 Å of N5 of the FAD
that is in perfect hydride transfer distance
The edge-to-edge distance between the C8M of the FAD and the proximal Fe of the [2Fe−2S] cluster is 9.4 Å
The adenine moiety of NADH resides in a separate pocket of the protein
whereas the nicotinamide shares a pocket with the isoalloxazine of FAD
In contrast to the cryo-EM structure the X-ray structure of isolated NqrF in complex with NADH the nicotinamide is separated from the isoalloxazine by Phe406 and cannot transfer its hydride to N5 of FAD
Residue Phe406 has to move out of the binding pocket to promote hydride transfer
To address the role of residue Phe406 in NADH binding
we determined the X-ray structure of a NqrF variant where Phe406 is replaced by Ala
In contrast to wildtype NqrF the NqrF Phe406Ala variant exhibited productive binding of the nicotinamide moiety of NADH in close proximity to the FAD
The structure revealed that the nicotinamide binds close to the isoalloxazine
The C4N of the nicotinamide group of NADH is in a distance of 3.5 Å of N5 of the FAD
X-ray structure of NqrF subunit in complex with NADH shown in a similar orientation like in c
The 2fo-fc at 1.5 σ around bound NADH is shown
The hydrophilic domain of NqrC moves between two positions at either NqrB or NqrD-E shuttling the electrons from the intramembranous [2Fe−2S] in NqrD-E to NqrB
The cryo-EM structures and the X-ray structures represent snapshots of these switching movement of NqrC
NqrB and NqrD which are predicted to form disulphide bonds in either state
The cysteine residues are located in the periplasm that with its oxidizing environment facilitates disulphide bond formation
Variants of Na+-NQR with corresponding cysteine residues were isolated and analysed by non-reducing SDS-PAGE
Both variants corresponding to both states of NqrC form disulphide bonds as indicated by the shift of bands to higher molecular mass
The covalent FMN containing subunits NqrC and NqrB were monitored by their fluorescence at 508 nm
The disulphide crosslink of NqrC with NqrB and with NqrD demonstrates that both conformations occur in vivo
Both variants showed diminished ratios of UQ-1/NADH reduction rates showing that the electron transfer through Na+-NQR is impaired
Reduction of the disulphide bonds restores the electron transfer to UQ-1
as shown by an approximate 2-fold increase of the UQ-1/NADH ratios
Kinetic data are shown as mean ± SD including error propagation
Individual data points are shown as open spheres
Two-sided paired sample t test was applied with confidence interval = 0.95 and degree of freedom =6
5.71 10−5 for variant NqrC-P174C-NqrD-Q100C
and 0.003 for variant NqrC-L226C-NqrB-P376C
Vibrio cholerae strains expressing the variants instead of wt Na+-NQR are drastically impaired in growth displaying slower growth rates and 45% lower cell yields
n = 3 biologically independent experiments
Source data
NqrB (orange) contains a covalent FMN and a riboflavin as cofactors
Both flavins are depicted as yellow spheres
Detailed view on the location of FMN and riboflavin in NqrB
The FMN cofactor is located close to the periplasmic aspect of NqrB
the riboflavin closer to the cytoplasmic aspect
Interactions of riboflavin with the residues of NqrB
Several hydrogen bonds (green dotted lines) are formed with the ribityl sidechain and the isoalloxazine
The backbone amide of Gly198 and the sidechains of Asn200
and Asp346 form hydrogen bonds with the oxygen atoms of the ribityl chain
The backbone amide and carbonyl of Ala205 and Phe342 as well as the sidechains of Thr162 and Asn203 form hydrogen bonds with N1
Voltage generation by isolated wt Na+-NQR and variant Na+-NQR-NqrB-D346A
Voltage generation by the variant is drastically decreased
Growth of Vibrio cholerae expressing either wt Na+-NQR (■)
or a Na+-NQR variant lacking the entire subunit NqrB (○)
Growth rate and growth yield of Na+-NQR-NqrB-346A variant (▲) is diminished
Source data
UQ-1 is interacting mainly with hydrophobic residues of NqrB
One hydrogen bond is formed to the backbone carbonyl oxygen of Asn156
Cryo-EM map around inhibitor HQNO (magenta)
HQNO interacts with similar residues like UQ-1
HQNO forms two hydrogens bonds with backbone amide of residues 159 and 160 or NqrB
HQNO binds somewhat deeper into NqrB than ubiquinone
The residues NqrB155–157 shift by about 1.5 Å creating a slightly larger binding pocket than the ubiquinone
HQNO recruits the N-terminal amphiphilic helices to form a high affinity binding site
Docking of UQ1 into the structure of Na+-NQR yields a solution that is reasonable agreement with the modelled UQ-1
Docking of HQNO into the structure of Na+-NQR gives a perfect match of the docking solution and the modelled HQNO
that is HQNO is predicted to bind with higher affinity than UQ-1
Cross section through subunits NqrD-E at the position of the [2Fe−2S]NqrD-E (shown as spheres)
The cryo-EM structure of NqrD-E in the oxidized state is shown on the left-hand side in dark colors
The structure assigned to a reduced [2Fe−2S]NqrD-E cluster is shown on the right-hand side in light colors
The distances of the cluster to the membrane planes are indicated
the cluster moves almost 2 Å relative to the membrane plane
Structural alignment of NqrD-E and of the NqrC
The conformational changes are indicated by arrows
illustrating how NqrD-E opens in the oxidized state (dark colors) compared to the reduced state (light colors)
Detailed view of structural changes in the region of helices III and IV of NqrD-E
The movement of the helices between both states is indicated by arrows
NqrD-Arg71 of and NqrE-Glu95 approach each other to form a salt bridge stabilizing the conformation corresponding to the reduced state of the [2Fe-2S]NqrD-E cluster
Anomalous difference maps in the region of entire Na+-NQR
The map is derived from crystals grown in the presence of CsCl
The dataset was recorded at 1.7 Å close to the L-I edge of Cs to maximize the anomalous contribution of these metal ions
the [2Fe-2S]NqrD-E and rigidly bound Cs+ will exhibit a strong anomalous signal
Strong anomalous difference map peaks (green) are observed at the positions of [2Fe-2S]NqrF
[2Fe-2S]NqrD-E and at the periplasmic aspect of NqrB
Anomalous difference maps of Na+-NQR derived from crystals grown in the presence of RbCl
The dataset was recorded at the K-edge of Rb at 0.82 Å
Strong anomalous difference map peaks (red) are observed at the periplasmic aspect of NqrB
Some minor peaks deriving from the [2Fe-2S] clusters are observed as well
Overlay of the anomalous difference maps deriving from Cs+ (green) and Rb+ (red) bound to Na+-NQR
The binding site for both ions maps to site Na-2 close to the interaction site of NqrB with NqrC
Na+-dependent NADH oxidation rates of wt Na+-NQR and variants NqrB-F338A and NqrB-F342A
The variant exhibits an NADH oxidation rate that is about 5% diminished compared to wt Na+-NQR
whereas variant NqrB-F342A shows a 7% higher activity than wt NQR
Na+-dependent UQ1 reduction rates reveal almost identical rates for wt Na+-NQR and variant NqrB-F342A
while the rate for NqrB-F338A is reduced by about 8%
electron transfer activity is only marginally affected in both variants confirming that the structural integrity is not affected by these mutations
Voltage generation in proteoliposomes monitored with oxonol is reduced by about 30% for variants NqrB-F338A and NqrB-F342A compared to wt Na+-NQR
Residues Phe338 and Phe342 are located at the constriction of the proposed Na+-translocation pathway and might serve as a gate
In both variants the bulky Phe residue has been replaced by the smaller Ala
This may be explained by a backflow of Na+ during translocation because of an incomplete closure of the gate
In control experiments without addition of NADH (dotted trace)
Source data
Kinetics and coupling of wildtype Na+-NQR and variants with engineered disulfide bonds; growth curves of wildtype Na+-NQR and variants
Unprocessed Coomassie-stained gel and flavin fluorescence of gel
Voltage generation by wildtype Na+-NQR (wildtype is same as in Extended Data Fig
10) and Na+-NQR variants NqrB-D346A; growth curves of wildtype Na+-NQR and variant NqrB-D346A
Kinetic characterization and voltage generation by wildtype Na+-NQR (voltage generation of wildtype is same as in Extended Data Fig
5) and Na+-NQR variants NqrB-F338A and NqrB-F342A
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was the lead scientist for first human trial substituting refined sugars with pure maple syrup
The study found significant improvement in multiple cardiometabolic risk factors.
Quebec, CA, November 18, 2024 – A new study published in the The Journal of Nutrition
found that substituting two tablespoons of pure maple syrup for refined sugars reduced several cardiometabolic risk factors in humans. It was the first placebo-controlled clinical trial exploring potential health benefits of maple syrup in humans
“We know from decades of research that maple syrup is more than just sugar. It contains over 100 natural compounds, including polyphenols, that are known to prevent disease in part through their anti-inflammatory effects,” remarked Dr. André Marette, PhD
“Because the fundamental chemistry of maple syrup is unique
I wondered if ingesting maple syrup instead of an equivalent amount of refined sugar would differently impact the cardiometabolic health and the intestinal microbiota in humans. The results were extremely encouraging
I did not expect to see so many improvements of risk factors within a relatively short treatment period.”
The study was conducted by a Laval University team led by Dr
at the Quebec Heart and Lung Institute and Dr
at the Institute of Nutrition and Functional Foods
Forty-two volunteers from the greater Québec city area
Participants substituted 5% of their daily caloric intake (corresponding to 2 tablespoons) from refined sugars with either Canadian maple syrup or an artificially flavored sucrose syrup
Each phase lasted 8 weeks with participants switching between maple syrup and sucrose syrup groups after a four-week washout period. The cross-over design ensured that the same test subject was his or her own control
Primary outcomes focused on the oral glucose tolerance test
the OGTT. Secondary outcomes included changes in blood lipid profile
body fat composition (measured by DEXA scan) and changes in gut microbiota composition
Improves Multiple Cardiometabolic Risk Factors
Study participants who consumed pure maple syrup had an improved response to the oral glucose tolerance test (OGTT) than those who received a flavored syrup of refined sugar. Their bodies managed blood sugar levels better after eating (-50.59 vs
Blood pressure was also lowered in the subjects who consumed maple syrup during the trial
Systolic blood pressure decreased significantly in the maple syrup group (-2.72 mm Hg) while it increased slightly in the sucrose group (+0.87 mm Hg)
“Lowering blood pressure continues to be an important factor in lessening the risk of cardiovascular disease,” Dr
can be part of an overall solution in helping to prevent metabolic diseases.”
Visceral fat is the deep fat that wraps around the internal organs in your belly. It can increase an individual’s risk of serious health problems such as heart disease
The maple syrup trial showed that android fat mass
significantly decreased in the maple syrup group as compared to an increase in the group consuming the sucrose solution (-7.83 g vs
An unexpected discovery was the improved levels of potentially beneficial gut bacteria and a decrease in levels of potentially harmful gut bacteria in the maple syrup participants
The study showed a reduction in Klebsiella species and Bacteroides pectinophilus
which are linked to inflammation and metabolic disorders
and the increased growth of beneficial bacteria like Lactocaseibacillus casei and Clostridium beijerinckii
the study findings are quite significant,” Dr
Marette noted. “The combined decrease of such key risk factors may help to reduce the risk of diabetes and cardiovascular disease
Making a commitment to lifestyle changes and small adjustments to our everyday diets is important and can be a powerful tool in preventing future diseases.”
According to one participant: “Before the study
I would consume pure maple products regularly but not consistently
Today my routine is to replace refined sugars with 2 tablespoons of pure Canadian maple syrup daily.”
First Human Trial Builds Upon American Researcher’s Cellular and Animal Studies
Dr. Marette’s clinical study builds upon his own work in animal models of diabetes and previous work on maple syrup and its bioactives by American scientist Navindra P. Seeram, PhD
Seeram’s extensive foundational work with maple syrup set the stage for this first human clinical trial
we learn more benefits that natural products from medicinal plants and functional foods
“The significant promising results of this first human trial provide more reasons for us to educate consumers about maple syrup’s many health benefits
It is truly a ‘smarter sweetener’ and a healthier alternative to refined sugar.”
“While this study was limited to a relatively small sample size (42 men and women) and took place during a relatively short duration of time
the results are still significant,” Dr
“We now have human evidence to support replacing refined sugars with maple syrup
for preventing metabolic diseases. Our next goal is to conduct larger studies with other populations to explore how replacing refined sugars with maple syrup might impact their unique health conditions.”
General nutrition claims for 2 tablespoons of maple syrup:
The study was jointly funded by Québec Maple Syrup Producers and the Québec Department of Agriculture
Fisheries and Food (MAPAQ) through its healthy food production initiative
To find out more about this and other clinical studies about maple syrup, please visit ppaq.ca/en/medias/clinical-study.
The Québec Maple Syrup Producers (QMSP) represent over 13,500 maple producers and 8,400 maple enterprises
Québec produces 72% of the world’s maple syrup and exports it to over 70 countries.
# # #
10.1016/j.tjnut.2024.08.014
Substituting Refined Sugars With Maple Syrup Decreases Key Cardiometabolic Risk Factors in Individuals With Mild Metabolic Alterations: A Randomized
The study was jointly funded by Quebec Maple Syrup Producers and the Quebec Department of Agriculture
Fisheries and Food (MAPAQ) through its healthy food production initiative
are not responsible for the accuracy of news releases posted to EurekAlert
by contributing institutions or for the use of any information through the EurekAlert system
Copyright © 2025 by the American Association for the Advancement of Science (AAAS)
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four Bundeschampionate qualifiers took place in Germany
the winners were 5-year olds Gut Wettlkam's Evée and Elodie
and the the 6-year old Djamalla and Special Gold PCH
Eleven horses competed in the L-level test for 5-year olds
Johanna Wadenspanner topped the board with Gut Wettlkam's DSP mare Evée (by Escolar x San Amour) on a score of 8.2
and 8.5 for submission and general impression
Eilika Böye and Evolution Dree Böken (by Escolar x Lauries Crusador xx) followed in second place with 8.0
The Rhinelander gelding is owned by the Werndl family and got 8 for walk
7 for submission and 8 for general impression
The M-level dressage horse test for 6-year olds featured 8 pairs and Franz Trischberger and Therese Mercker's Oldenburg mare Djamalla (by Don Romanov x Sir Donnerhall) bested the field with 8.2
Ina-Marie Blass and her own Hanoverian stallion Farrokh (by Finest x Hotline) were second on 8.0 after the black got 8.5 for walk
7.5 for submission and 8.5 for general impression
At the qualifier in Vöhl the L-level dressage horse test for 5-year olds had eight combinations at the starters line
and Dorothee Lehan rewarded the high score of the class to Katharina Hemmer aboard Gut Neuenhof's Westfalian mare Elodie (by Escolar x Soliman de Hus)
They won the class with 8.3 and edged out Claudia Rassmann on Johannes Schmidt's Oldenburg mare Habibi (by For Romance x Dimaggio) with 8.2
The 6-year old class was judged by Ute Kombächer
Dieter Scheermann and Elke Hüther and they rewarded Katharina Hemmer a whopping 9.0 for the victory aboard Nancy Gooding's Oldenburg stallion Special Gold PCH (by San Amour x Don Schufro)
Philipp Hess and Norma Klemstein's Hanoverian stallion followed in their wake in second place with 8.3
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The tragic and instant collapse of the Francis Scott Key Bridge in Baltimore in the early hours of Tuesday
after a cargo ship apparently lost power and consequently lost steering
causing it to ram into one of the bridge supports
is an example of how most catastrophes occur: a series of smaller events align to create the disaster that causes harm.
My background as a sailor, along with my experience working in the Electric Boat division of General Dynamics
helps me understand some of the details surrounding the accident
My position at Boston University’s Questrom School of Business as an operations professor who studies human error and accidents also gives me some unique insight
The organizations involved reflect the nature of today’s global supply chains
which is owned and operated by Singapore’s Synergy Marine Group
to ship its customers’ goods to Sri Lanka via a monthlong voyage
There were two local “harbor pilots” on board
who are experts in the specific harbor and who are responsible for safely navigating ships in and out of the busy Baltimore harbor
Cause: The ship seemed to have an electrical problem (as evidenced by the loss of lights two times before the collision
The loss of power meant that the pilots were drifting
Smoke was seen rising from the boat as it struck the bridge support
suggesting they were logically trying to reverse the boat
The current and wind conditions blew the boat into one of the Francis Scott Key Bridge’s support structures at 1:26 am
The boat was going about 8 knots due to the current
Response: The ship’s crew called Maryland’s Department of Transportation and issued a mayday call to the US Coast Guard moments before the crash
which enabled the Department of Transportation to stop traffic going onto the bridge
Maryland’s governor called those who stopped additional traffic from entering the bridge after the mayday call “heroes.”
Impact on supply chains: The bridge collapse will have a negative impact on the timeliness of delivery of several important goods
Ten commercial ships that were headed into Maryland’s port have been forced to anchor outside the harbor
Up to 40 shipping vessels are en route to the Port of Maryland and will also likely be affected
The Port of Maryland is the 11th busiest port in the US and handles imports of cars
the Port of Maryland handled 750,000 vehicles
the highest of all US ports in terms of vehicles
Maersk’s stock was down 2 percent after the announcement of the accident
Prevention: The bridge was built in 1970 and is a “truss” type of bridge with no redundancy to compensate for the loss of a support structure
It’s important to note that cargo ships are now two times larger than cargo ships in the 1970s
increasing the probability and risk posed by them striking a bridge due to the vessels’ large mass and size
the Port of Maryland does not require exiting and entering cargo ships to be escorted by tugboats
which could have towed the Dali to safety when it lost its steering ability
it seems clear that having tug escorts or availability of tugs seems prudent
or adding additional support for vulnerable bridges
I suspect the cost of taking these measures seemed prohibitive given the low probability of a ship striking the bridge
it is unclear whether there were systematic problems
It has been inspected 27 times since it was built in 2015
an inspection in Chile listed a deficiency related to the propulsion and auxiliary machinery—gauges
the deficiency was corrected the same day and the last inspection
We should ask whether similar problems could happen at other ports
Synergy Marine Group’s Founder and Executive Chairman Captain Rajesh Unni warned that current port infrastructure is misaligned with today’s shipping vessels
this tragedy is typical of how most accidents occur
Rather than being caused by a single mistake or human error
a series of minor issues align catastrophically to cause human harm
The ship lost power (issue 1) as it was leaving the port before it passed under the bridge (issue 2)
strong winds and currents (issue 3) blew it into the bridge
which was an old bridge (issue 4) with insufficient support to withstand losing one of its pillars (issue 5)
and the Port of Maryland did not require tug assistance
so there was no back up for the boat itself when it lost steering (issue 6)
All those elements had to be present for the ship to strike the bridge
if the ship had lost steerage after clearing the bridge
or if the currents were not as strong as they were
or if tugboats had been required to help guide the ship
it’s probable this would have been just a “near-miss” incident
The challenge for organizations and governments is to respond to near-miss incidents by taking measures to prevent future accidents that might have worse outcomes
Anita Carson is Larz Anderson Professor in Operations & Technology Management and department chair of operations and technology management at BU’s Questrom School of Business
“POV” is an opinion page that provides timely commentaries from students, faculty, and staff on a variety of issues: on-campus, local, state, national, or international. Anyone interested in submitting a piece, which should be about 700 words long, should contact John O’Rourke at orourkej@bu.edu
BU Today reserves the right to reject or edit submissions
The views expressed are solely those of the author and are not intended to represent the views of Boston University
POV: Was the Francis Scott Key Bridge Disaster Avoidable
Should the cargo ship have been traveling more slowly
Reversing port (left) stern will turn bow to the right toward the bridge support as the inertia from the weight of the boat continues forward into the pylon
Reversing starboard (right) i believe would have opposite effect
Beyond all this i believe they have bow thrusters to prevent such issues
Furthermore i am sure they have alarms going off when they are off their shipping route especially approaching bridges when caprains and his bridge crew should all be paying attention
As far as wind and currents being too strong this boat would be clearly in a different position more parallel to the bridge than it was currently in after the impact
Power going off at the most critical time is like someone winning the mega lotto
It would be very valuable to get some experienced captains in commercial freight their comments rather than opinions from talking heads on news channels
Agree completely with this very important post
Consider that the Dali was in the channel and properly aligned before the electrical occurrence
The Dali was diverted from her vector of trajectory
The likeliest cause was human activity such as dropping anchor and effectuating some mechanical steering
Engineering must provide for a large margin of shocking human error
which is sometimes enhanced by distraction
Tug Boats should be required – in the future unfortunately – from point of docking (which they are in this port) past the Bridge to harbor entrance
This clearly laid out all of the issues surrounding this tragedy in an interesting and succinct fashion
Now let us pray for the six souls lost yesterday morning
This disaster will influence managers’ future decisions when dealing with risks of great consequences
I would agree wind and current had little or nothing to do with the incident
It will be easy enough to tell whether reversing that ship’s engine at high revs would cause the boat to turn the way it appears to turn in the video
It’s quite possible the ship has a single screw that rotates clockwise in forward
Kicking to port in reverse would be the expected result
A tug standing by near the bridge abutment could have pushed the hull in a way that would have steered it away from the bridge without actually being attached to the Dali
I’m guessing the statistical possibility of a ship losing steerage entering or leaving a commercial port is negligible
They don’t prepare for it because thousands of transits in and out of commercial harbors around the world have never produced this same result
It appears at least one of them helped alert law enforcement and saved lives
Two pilots onboard means you have at least three people on the bridge potentially acting as captain
I have no other facts to support this opinion but I could imagine in a moment of panic three people not used to working as team members could end up working at cross purposes
Certainly they would have been usinh all means available to avoid collision
Thrusters are less then effective abive three knots
I cant imagine she bleed off any more the three knots before the collision
There is no mention in the article of the lack of passive protection of the bridge pillars
Around the time of the construction of the Baltimore bridge a much smaller vessel hit and demolished the Sunset Skyway Bridge over Tampa bay
As a result legislation was written that physical barriers to prevent contact between vessels and bridge supports should be included in all new bridge design but there was no requirement to fit protection retrospectively
Four small protective dolphins were installed but they would only stop a rowing boat
some by seemingly qualified civil engineers
that claim that the presence of many dolphin protections on each side of the bridge would NOT have stopped a ship as big as the Dali
While not a professional civil engineer today
I did study civil engineering in college performed did many computerized structural analyses of various structures
There is zero doubt in my mind that a system of dolphins on both sides of the bridge would have prevented the collapse if not also major structural damage
It’s simply a matter of how many and how large they would need to be
the Dali was stopped by the pier structure holding up the main support
so a dolphin of that size would clearly have worked
but far less than the cost of rebuilding that bridge and paying the wrongful death settlements that will arise from this tragedy
Enough already with the “dolphins would not have prevented this” talk
Let’s identify all similarly vulnerable bridges and start protecting them
Pioneering Research from Boston University
Castelblanco, 42, of Huntington Beach, was diagnosed with leukemia in 2010 and received a bone-marrow transplant from Vohl, 41, of Stuttgart, Germany, months after her diagnosis.
Three years later, the women who didn’t know one another learned they now share a blood type — and some DNA.
“Before, I was A-positive, and now I’m B-positive,” Castelblanco said about her changing blood type, as Vohl simultaneously finished the sentence. “And my [bone marrow] DNA is hers. So in the inside, we’re the same.”
Tears were shed as Castelblanco, along with her family and friends, gathered at Lake Park in downtown Huntington Beach on Saturday to visit with the woman who saved her life.
Delete Blood Cancer DKMS, a New York-based nonprofit that registers donors from around the world and transports bone marrow for transplants, helped organize the afternoon get-together and flew Vohl and her son out to California for a week.
“This is a celebration, not only to introduce Yvonne to everyone, but also to thank everybody here for everything that they’ve done,” Castelblanco said.
Vohl said she wouldn’t have organized such a large event to announce her arrival, but was humbled by the thanks she received from Castelblanco’s family and friends.
“They told me that I’m a hero and that they wanted to bow down [to me],” Vohl said.
Monica Pavalko and Shelley Phillipps, friends of Castelblanco, said they’ve been by her side since Day One, helping her with chores and taking care of her family.
The two said her strong will and determination is what has kept her going for the past three years.
“She never complained or asked, ‘Why me? This sucks,’” Phillipps said. “You felt like you couldn’t cry in front of her. She always said, ‘I’m going to beat this. I’m good.’”
On April 22, 2010, Castelblanco was diagnosed with acute myeloid leukemia, a form of cancer that lowered her blood cells and substantially lowered her immunity, said Dr. Vinod Pullarkat, her physician at USC Norris Cancer Hospital.
A month before her diagnosis, Castelblanco was participating in a half-marathon in Florida. She said she wasn’t doing well in the run and thought she was tired or hadn’t trained enough.
“We got home, and I just kept making excuses for why I wasn’t feeling well,” Castelblanco said. “I was saying I had the flu, or maybe I was pregnant, and all these things as to why I wasn’t doing well.”
She was admitted to Hoag Hospital in Newport Beach and underwent a round of chemotherapy, but the leukemia cells were not responding to the treatment, Pullarkat said.
Upon further inspection, Castelblanco was discovered to have an aggressive form of leukemia, and the only viable treatment would be a bone-marrow transplant.
With advancements in medicine and technology, 70% of patients with acute myeloid leukemia have a chance at surviving, Pullarkat said.
In Castelblanco’s case, however, there was a slim success rate.
Castelblanco was transferred to City of Hope National Medical Center in Duarte, where Pullarkat was working at the time. The search for a bone marrow donor began immediately with Pullarkat trying to find matching tissue types.
Family members were tested, but no one was a match. So Pullarkat turned to the world registry to see if anyone could be a near-perfect donor for his patient.
Vohl was 25 years old when she registered herself as a bone marrow donor, she said.
The company she was working for put together a registry drive with DKMS, offering time off work and lunch to the employees who joined.
Years passed, and Vohl didn’t receive a phone call from the company. Then, in August 2010, she was contacted and told she was a match for someone in the United States.
She said she didn’t think twice about donating her bone marrow.
“My company gave me holidays,” Vohl said. “DKMS booked the hotel and plane and organized everything.”
The Stuttgart resident was flown to Dresden, where doctors checked her physical condition. Once she was cleared, she was given injections to increase her blood count for about five days and was hooked to a machine that would collect stem cells from her blood through an IV rather than from her hip, Vohl said.
“It was just two needles [in my arms] and a big machine behind me,” she said. “It wasn’t painful. It was like donating blood. It takes a little bit longer, but it was so easy.”
The traditional way to harvest bone marrow was to sedate the donor and collect the cells from the hip, Pullarkat said.
But for the past 20 years, doctors have been extracting stem cells through the donor’s blood.
“It made the donations much easier,” Pullarkat said. “Bone marrow harvesting is still done, but the majority of the transplants nowadays are done by using blood stem cells. The end result is the same: They both go in the bone marrow, and they will produce new blood.”
Those stem cells were then injected into Castelblanco so that her body could begin producing new blood, Pullarkat said. And since the cells are from Vohl, Castelblanco’s blood type changed and her bone marrow DNA matches her donor’s.
Castelblanco received the bone-marrow transplant on Sept. 2, 2010, but she still wasn’t in the clear.
“You get very sick for a while,” she said. “The first 100 days, post-transplant is a very critical time. Once you get through that magical 100 days, then every month that you stay healthy, your chances [of surviving] become better.”
She didn’t stay in the hospital long after her transplant. Castelblanco said she was released 28 days after the procedure, which is better than most patients, but she still had to deal with the side effects of her transplant and medication.
Castelblanco developed a cataract in her right eye and experienced some intestinal issues and discoloration of her skin because of graft-versus-host disease (GVHD).
“It’s just the new system attacking my body and trying to work on finding its new home,” Castelblanco said. “A lot of my medication is to prevent attacks on my organs and things like that.”
Pullarkat said Castelblanco’s case of GVHD isn’t life-threatening and is managed through medication. Because her leukemia is in remission, he considers the transplant a success.
Because of privacy and other issues, Castelblanco and Vohl had to wait for two years after the transplant to get each other’s contact information.
“It’s to protect the patient and the donor,” Castelblanco said. “I could have had the transplant and still not have done well and maybe not lived. How could you not have a relationship with the person that saved your life? But if you don’t do well, it could have a [negative] reflection on them.”
Castelblanco’s dream during those two years was to get ahold of Vohl as soon as she could to thank her. But as soon as she got her contact information in September 2012, Castelblanco didn’t know what to say.
“‘Thank you’ just doesn’t sound like enough,” she said. “It so hard to type that emotion in an email, but I think we understood each other.”
Castelblanco said she is still under supervision and continuing to recover.
She had cataract surgery Aug. 12, and the color in her skin is slowly returning to normal.
Vohl said she’s getting a tour around Southern California and will be visiting Disneyland and Hollywood.
And once she becomes healthier, Castelblanco said she’s planning to go to Germany to visit Vohl in her home country.
“Life just goes on,” Castelblanco said. “You just look at the positives every day, and if something were to reoccur, you just deal with it.”
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Volume 9 - 2022 | https://doi.org/10.3389/fnut.2022.740898
This article is part of the Research TopicMobile Health and NutritionView all 4 articles
Machine learning (ML) algorithms may help better understand the complex interactions among factors that influence dietary choices and behaviors
The aim of this study was to explore whether ML algorithms are more accurate than traditional statistical models in predicting vegetable and fruit (VF) consumption
A large array of features (2,452 features from 525 variables) encompassing individual and environmental information related to dietary habits and food choices in a sample of 1,147 French-speaking adult men and women was used for the purpose of this study
was measured by averaging data from three web-based 24 h recalls and used as the outcome to predict
Nine classification ML algorithms were compared to two traditional statistical predictive models
logistic regression and penalized regression (Lasso)
The performance of the predictive ML algorithms was tested after the implementation of adjustments
as well as in a series of sensitivity analyses such as using VF consumption obtained from a web-based food frequency questionnaire (wFFQ) and applying a feature selection algorithm in an attempt to reduce overfitting
Logistic regression and Lasso predicted adequate VF consumption with an accuracy of 0.64 (95% confidence interval [CI]: 0.58–0.70) and 0.64 (95%CI: 0.60–0.68) respectively
the most accurate algorithms to predict adequate VF consumption were the support vector machine (SVM) with either a radial basis kernel or a sigmoid kernel
both with an accuracy of 0.65 (95%CI: 0.59–0.71)
The least accurate ML algorithm was the SVM with a linear kernel with an accuracy of 0.55 (95%CI: 0.49–0.61)
Using dietary intake data from the wFFQ and applying a feature selection algorithm had little to no impact on the performance of the algorithms
ML algorithms and traditional statistical models predicted adequate VF consumption with similar accuracies among adults
These results suggest that additional research is needed to explore further the true potential of ML in predicting dietary behaviours that are determined by complex interactions among several individual
despite several public health efforts and policies
adhering to healthy eating remains a challenge
the present study is one of the first to compare ML algorithms to traditional statistical models to predict a dietary behavior
the aim of this study was to explore and compare the performance metrics of ML algorithms and traditional statistical models to predict a simple healthy dietary behavior
adequate vegetable and fruit (VF) consumption
We hypothesized that ML algorithms are more accurate than traditional statistical models in predicting adequate VF consumption
We stress that this analysis was not intended to provide a definitive predictive model of adequate VF consumption
Once all questionnaires had been completed
participants were invited to their regional's research center for clinical assessment (anthropometric measurements and blood sampling)
The project was conducted in accordance with the Declaration of Helsinki and was approved by the Research Ethics Committees of Université Laval (ethics number: 2014-271)
Centre hospitalier universitaire de Sherbrooke (ethics number: MP-31-2015-997)
Montreal Clinical Research Institute (ethics number: 2015-02)
and Université du Québec à Trois-Rivières (ethics number: 15-2009-07.13)
The set of predictor variables and their corresponding features were derived from all questions and scores from all questionnaires listed in Supplementary Table 1
A variable represented a question in a given questionnaire
while its corresponding features reflected the transformed variable
dummy variables for each response to that question
fasting blood glucose and insulin concentrations
systolic and diastolic blood pressures were also considered as features in each model and algorithm
body fat percentage and waist circumference were considered as features in all models and algorithms
Questions that had been completed by <70% of the participants were excluded
Missing data for continuous features were imputed using the study population averages for each feature
The categorical variables were dummy coded with a specific binary code for missing data
Once categorical variables were dummy coded
total number of predictor features included on all models and algorithms was 2,452
The outcome predicted (classes) was VF intake dichotomized as adequate/inadequate, based on the population target in Québec of 5 or more servings/d (27)
the two classes were 1- adequate VF consumption
corresponding to 5 or more servings/d and 2- inadequate VF consumption
the list of discriminant features retained in the LR
SVM linear and Adaboost models and algorithms were compared to verify any similarities or differences
The discriminant analysis was conducted by identifying the 10 features with the highest coefficients for LR
Gini feature importance was used for the discriminant analysis of the RF and Adaboost algorithms
and Entropy importance was used for the DT algorithm
All features retained by the SCM corresponded to the discriminant features for this algorithm
KNN does not rank features based on importance and SVM (polynomial
radial basis and sigmoid) are uninterpretable
data from these algorithms were not included in the discriminant analysis
Predictive metrics and corresponding equations
Table 3 shows characteristics of the 1,147 participants (572 women
The majority of participants had a university degree and were Caucasian
The mean (±standard deviation) VF consumption evaluated by the R24W in the sample was 5.5 ± 3.1 servings/d (interquartile range = 4.0)
with 52.3% of participants consuming 5 or more servings/d
The mean VF consumption evaluated by the wFFQ was 7.6 ± 5.0 (interquartile range = 4.8) with 67.6% consuming 5 or more servings/d
Sociodemographic characteristics of the French-speaking adults from Quebec
Table 4 presents the metrics of all models and algorithms predicting adequate VF consumption (≥5 servings/d) based on normalized data among all participants
There are no significant differences in accuracy between models and algorithms and no important differences for other performance metrics
When predicting inadequate VF consumption (<5 servings/d) instead of adequate VF consumption
there were no differences in performance between traditional statistical models and ML algorithms (not shown)
Performance metrics of two traditional statistical models and nine machine learning algorithms to predict adequate vegetable and fruit (VF) consumption based on dietary intake data obtained from web-based 24-hr recalls (R24W) among1147 French-speaking adults from Québec
Figure 1 presents the top discriminant features included in seven of the classification models and algorithms. Discriminant features are colour-coded for illustrative purposes to allow rapid visual comparison. Figure 1 shows that the discriminant features predicting adequate VF consumption are inconsistent across models and algorithms
While the traditional classification models LR and Lasso shared eight top discriminant features
there is little coherence between the discriminant features of the five ML algorithms
No single feature was included as a top discriminant feature in all seven models and algorithms
Discriminant features retained in the logistic regression (LR) and Lasso models and in the decision tree (DT)
support vector machine (SVM) with a linear kernel and Adaboost machine learning algorithms to predict adequate vegetable and fruit consumption
Features are colour-coded according to the questionnaire to which they belong; different shades within a given color indicate that more than one feature of a questionnaire was retained; numbers indicate the rank of a given question from a given questionnaire retained in the model or algorithm
Social support for healthy eating questionnaire; BIDR
Balanced inventory of desirable responding; FLQ
Sensitivity to punishment and sensitivity to reward questionnaire
sensitivity and F1 scores were also higher when using intake data from the wFFQ compared to data from the R24W
AUROC values for all models and algorithms were lower when using data from the wFFQ compared to data from the R24W
except for the Lasso model for which the AUROC value slightly increased
Performance metrics of two traditional models and nine machine learning algorithms to predict adequate vegetable and fruit (VF) consumption based on dietary intake data obtained from a web-based food frequency questionnaire (wFFQ) among1147 French-speaking adults from Québec
The accuracy of traditional statistical models and of ML classification algorithms increased when dietary features known to be correlated with VF consumption were included in the analyses (Figure 2). Other performance metrics are reported in Supplementary Table 4
Accuracy of the various ML classification algorithms in predicting adequate VF consumption was once again not superior to accuracy seen with traditional statistical models
Comparing the accuracy of traditional statistical models and machine learning algorithms to predict adequate vegetable and fruit (VF) consumption when other dietary intake features are included in addition to the 2452 features originally included
as well as components of the Canadian Healthy Eating Index (C-HEI) other than the VF component and the C-HEI score itself
Finally, reducing the number of features to 5, 10, and 50 features with a feature selection algorithm attenuated overfitting for most models and algorithms, but had trivial and inconsistent impacts on accuracy values and other metrics (Supplementary Figure 2; Supplementary Table 5)
the accuracy of all models and algorithms remained low
and no differences were observed between traditional statistical models and ML algorithms when fewer features were used to predict an adequate VF consumption
The successful use of ML in several healthcare fields suggests promising applications in the field of nutrition epidemiology and public health nutrition. However, the superiority and advantages of ML-based classification approaches compared with more traditional statistical approaches need to be evaluated, validated, and confirmed in all fields of application (3, 12, 37)
The objective of this study was to compare the performance metrics of ML algorithms to those of more traditional statistical models in predicting a tangible and simple dietary behavior
The hypothesis that ML classification algorithms outperform traditional statistical classification models when predicting adequate VF consumption based on a wide spectrum of individual
social and environmental data was not supported by our experimental data
accuracy of all models and algorithms increased when dietary intake data from the wFFQ were used in place of data from 24-h recalls
VF consumption measured over longer periods of time
and may therefore be more stable than when measured using average data from three 24-h recalls
this did not materialize into better performance metrics of ML classification algorithms compared to traditional statistical models
The fact that food frequency questionnaires are more prone to systematic error than 24-h recalls apparently did not negatively influence performance metrics of traditional statistical models and of ML classification algorithms
tended to slightly or substantially overfit despite normalizing the data from continuous features and adjusting hyperparameters to minimize overfitting and to optimize performances
Applying a feature selection algorithm to reduce the number of features included in the analyses lowered overfitting for all models and algorithms
accuracy improved for the majority of the models and algorithms when dietary features closely associated with VF intake were included
but overall performance of ML classification algorithms and traditional statistical models remained comparable
The compelling observation is that the ML classification algorithms tested in the present study do not predict adequate VF consumption with more accuracy than traditional statistical models when using a large set of features
Since the primary aim of this exploratory analysis was to compare predictive accuracy of different models and algorithms
multicollinearity did not have to be addressed
Future studies designed to identify discriminant features of adequate VF consumption or any other dietary behavior with traditional statistical models or with ML algorithms will need to consider multicollinearity
Our study also has the following strengths
this is the first study to compare ML algorithms with traditional statistical models to predict a dietary behaviour
We also used nine wellknown ML classification algorithms to conduct analyses
Algorithms showing strong predictive performances will have limited application if execution time is long
all algorithms used in this study had relatively short execution time
we included a rather large number of features
which could have allowed ML algorithms to capture non-linear and complex interactions
the number of features used may still be considered small according to some standards in the ML field
The extent to which ML classification algorithms outperform traditional statistical models when much larger and complex datasets are used to predict a dietary behavior outcome remains to be investigated
ML presents important opportunities for advancing the field of nutritional epidemiology and public health nutrition
our results suggest caution regarding the use and added-value of ML classification algorithms to predict diet-related variables and outcomes
in the context of predicting adequate VF consumption
ML classification algorithms did not perform better than traditional statistical models
Further research is needed to identify contexts for which ML algorithms are best suited
The raw data supporting the conclusions of this article will be made available by the authors
The studies involving human participants were reviewed and approved by Université Laval (Ethics Number: 2014-271)
Centre hospitalier universitaire de Sherbrooke (Ethics Number: MP-31-2015-997)
Montreal Clinical Research Institute (Ethics Number: 2015-02)
and Université du Québec à Trois-Rivières (Ethics Number: 15-2009-07.13)
The patients/participants provided their written informed consent to participate in this study
ÉC and DB contributed to some of the statistical modeling as well as to generating the data used in this study
and BL obtained funding for the PREDISE study
FL has contributed to the conceptualization of the analyses and the modeling
BL is the author responsible for this work
All authors contributed to the article and approved the submitted version
MC received a scholarship from the Fonds de recherche du Québec-Santé
The funding organisations were not involved in the writing of this article
The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest
All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations
Any product that may be evaluated in this article
or claim that may be made by its manufacturer
is not guaranteed or endorsed by the publisher
MCV is Tier 1 Canada Research Chair in Genomics Applied to Nutrition and Metabolic Health
The Supplementary Material for this article can be found online at: https://www.frontiersin.org/articles/10.3389/fnut.2022.740898/full#supplementary-material
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Laviolette F and Lamarche B (2022) Are Machine Learning Algorithms More Accurate in Predicting Vegetable and Fruit Consumption Than Traditional Statistical Models
Received: 13 July 2021; Accepted: 25 January 2022; Published: 17 February 2022
Copyright © 2022 Côté, Osseni, Brassard, Carbonneau, Robitaille, Vohl, Lemieux, Laviolette and Lamarche. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY)
distribution or reproduction in other forums is permitted
provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited
in accordance with accepted academic practice
distribution or reproduction is permitted which does not comply with these terms
*Correspondence: Benoît Lamarche, YmVub2l0LmxhbWFyY2hlQGZzYWEudWxhdmFsLmNh
Disclaimer: All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations
Any product that may be evaluated in this article or claim that may be made by its manufacturer is not guaranteed or endorsed by the publisher
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either observed and verified firsthand by the reporter
or reported and verified from knowledgeable sources
Translations may contain inaccuracies—please refer to the original content
"We know from decades of research that maple syrup is more than just sugar," Dr
that are known to prevent disease in part through their anti-inflammatory effects."
Metabolic disease is an umbrella term given to obesity and related diseases
A high-sugar diet and inflammation are two known risk factors for metabolic disease
and there has long been a debate among nutrition experts and scientists as to whether all forms of sugar are equally harmful to health
"Because the fundamental chemistry of maple syrup is unique
I wondered if ingesting maple syrup instead of an equivalent amount of refined sugar would differently impact the cardiometabolic health and intestinal microbiota in humans," said Marette
I did not expect to see so many improvements of risk factors within a relatively short treatment period."
and for eight weeks one group substituted 5 percent of their daily caloric intake of food with Canadian maple syrup
and the other group swapped the same amount of calories for artificially flavored sucrose syrup
there was a four-week washout period when the participants went back to their usual diets
before they spent another eight weeks eating the other sugar
This meant that the participants all experienced eight weeks eating each form of sugar
so the scientists could directly compare the effects of eating the equivalent of two tablespoons of Canadian maple syrup with two tablespoons of sucrose syrup
The scientists concluded that eating maple syrup rather than artificial syrup improved several markers of metabolic disease
their bodies afterwards responded better to the sugars in their blood
compared to when they ate the artificial syrup
Individuals in the maple syrup group showed significant improvements in blood pressure
while those in the sucrose group had higher blood pressure than on their regular diets
Abdominal fat is linked to an increased risk of heart disease
stroke and other metabolic conditions—but the scientists found that participants swapping their sugars for maple syrup lost abdominal fat
and those eating sucrose gained abdominal fat
the study findings are quite significant," said Marette
"The combined decrease of such key risk factors may help to reduce the risk of diabetes and cardiovascular disease."
"We now have human evidence to support replacing refined sugars with maple syrup
for preventing metabolic diseases," said Marette
"Our next goal is to conduct larger studies with other populations to explore how replacing refined sugars with maple syrup might impact their unique health conditions."
One of the study participants said in a statement: "Before the study
I would consume pure maple products regularly
Today my routine is to replace refined sugars with two tablespoons of pure Canadian maple syrup daily."
This study was published in The Journal of Nutrition. It was conducted by a team of scientists at Laval University
led by Marette at the Quebec Heart and Lung Institute
Marie-Claude Vohl at the Institute of Nutrition and Functional Foods
The research was partly funded by Quebec Maple Syrup Producers
which represents 13,500 producers of maple syrup and 8,400 maple enterprises
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Sheila Long is making a huge impact on students as a longtime school crossing guard
— A Weirton woman says it was her dream to be a teacher
And while you won’t find Sheila Long in a classroom
she's still making a huge impact on students as a longtime school crossing guard
you'll find her at the intersection of Euclid Avenue and Brightway along Marland Heights in Weirton
“People say I know their cars more than I know their faces,” she said
they say ‘I know who you are,’ and I say ‘what kind of car do you drive?’’’
Long sees to it that students make it safely off the bus and across the street
“Many times I've had to jump out of the way
‘listen to the rules because I don't want anything to ever happen to you.’’’
“I've had two (kids) graduate already
one is ready to graduate this year and one's a 4th grader
She's been wonderful,” parent Sharon Krutilla says of Long
Long gets a second helping of students at lunch time
as a cook in the cafeteria at Weir Middle School
Whenever I go up sometimes she comes around and gives me a hug to feel like I'm home or here getting off the bus
and it's just a really special feeling to me,” student Kylie Dean said
That special attention is appreciated by parents like Carlo Volhl
who waits for his 9-year-old son to get off the bus each day
which is thing we've been working for on while,” Vohl said
“A real feeling of community here with everybody
and it's nice to have someone like that on your side.”
And these kids know Long pulls out all the stops
She often takes the students for ice cream
“She has donuts in the morning and drinks for them
Long finds another special way to celebrate the kids hard work with water
and everyone brings water balloons and guns and we all have a water fight,” student Darren Thompson said
This week’s Shining Star is a charismatic crossing guard
finding ways to spread love with a little direction
and you just need to show them love and that makes me feel good,” Long said
“When I go home at night and lay my head on the pillow
and know I did what God wants me to do and these kids know their loved.”
Sheila is also a youth ministry leader in Weirton through the Awana organization and carpools kids to the program on a weekly basis
but says all the kids in her neighborhood are like her own
If you know someone, who goes above and beyond at their job, like Long, let us know. Nominate your Shining Star here
You could see them featured right here on NEWS9
NEW YORK (AP) - Disney has found its latest princess: 14-year-old native Hawaiian Auli'i Cravalho (aw-LEE'-ee crah-VOHL'-oh)
Cravalho was announced Wednesday as the star of Disney's upcoming animated adventure "Moana."
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Together with his criticisms of the Smithsonian representing un-American ideologies
Trump signed an Executive Order today demanding that the Nobel Prize committee abandon “woke and DEI” policies and grant prizes to people that really earn them
the Committee has granted prizes to undeserving recipients
Marie Curie should have never gotten one
She should return it and let someone else get the Peace Prize.”
He added that Barack HUSSEIN Obama didn’t do anything to deserve his
Look what I’ve done for the Ukraine.” Stephen Miller declared that it was the President’s intention that Oslo better shape up soon or we’d conquer Scandinavia
Peter Hegseth quoted on Signal. JD Vance was present for the signing and said
/satire (the foregoing is fictional and should not be taken for actual quotes)
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Metrics details
An Erratum to this article was published on 01 April 2005
Palmar xanthomas are characterized by a brownish, yellowish coloration of the palmar striae and are pathognomonic of type III dyslipidemia.
palmar xanthomas and features of type III (presence of β-VLDL
VLDL-cholesterol/TG ratio > 0.5) were observed among DM1-apo E2 heterozygotes individuals
DM1 individuals carrying the E2 allele (heterozygotes or homozygotes) tend to express palmar xanthomas
whereas unaffected apo E2 heterozygotes relatives do not
Our observations suggest that the simultaneous presence of DM1 and apo E2 allele promote type III expression
as shown by the familial evaluation of palmar xanthomas distribution
the search for palmar xanthomas while performing DM1 patients' physical examination might contribute to specify health status and identify the pattern of LD between DMPK and apo E loci
Patterns of linkage disequilibrium in the human genome
Cloning of the essential myotonic dystrophy region and mapping of the putative defect
Detection of an unstable fragment of DNA specific to individuals with myotonic dystrophy
Expansion of an unstable DNA region and phenotypic variation in myotonic dystrophy
Genealogical reconstruction of myotonic dystrophy in the Saguenay-Lac-Saint-Jean area (Quebec
The pleiotropoic expression of the myotonic dystrophy protein kinase (MDPK) gene illustrates the complex relationships between genetic
biological and clinical covariates of male aging
Type III hyperlipoproteinemia (dysbetalipoproteinemia): The role of apolipoprotein E in normal and abnormal lipoprotein metabolism
Linkage of myotonic dystrophy and apo E in a French-Canadian isolate
Myotonic dystrophy: Linkage with apolipoprotein E and estimation of the gene carrier status with genetic markers
Restriction isotyping of human apolipoprotein E by gene amplification and cleavage with HhaI
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This project was supported by the ECOGENE-21 project (CIHR/CAHR program grant no. CAR43283). D. Brisson is recipient of a doctoral studentship from the Canadian Institutes for Health Research (CIHR), Fournier Pharma, and the “Réseau en santé cardiovasculaire-FRSQ.” M.C. Vohl is a research scholar from FRSQ. D. Gaudet is the chairholder of the Canada Research Chair in preventive genetics and community genomics (http://www.chairs.gc.ca)
Montreal University Community Genomic Medicine Center and Chicoutimi Hospital Lipid Clinic Chicoutimi Hospital
Neuromuscular Diseases Clinic Jonquiere Hospital
Lipid Research Center and Department of Food Sciences and Nutrition Laval University
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DOI: https://doi.org/10.1097/01.GIM.0000157130.81975.FE
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a peroxisome proliferated activated receptor alpha (PPARα) agonist
has been shown to decrease plasma triglyceride (TG) and increase plasma high-density lipoprotein (HDL) cholesterol levels despite a large interindividual variation in the response
Fenofibrate-activated PPARα binds to a DNA sequence element termed PPAR response element (PPRE) present in regulatory regions of target genes
A PPRE has been identified in the proximal 5′ flanking region of the gene encoding the liver fatty acid binding protein (LFABP)
LFABP is a small cytosolic protein of 14 kDa present in the liver and the intestine and is a member of the superfamily of the fatty acid binding proteins (FABPs)
FABPs play a role in the solubilization of long-chain fatty acids (LCFAs) and their CoA-ester to various intracellular organelles
FABPs serves as intracellular acceptors of LCFAs
and they may also have an impact in ligand-dependent transactivation of PPARs in trafficking LCFAs to the nucleus
Since PPARs are known to regulate the transcription of many genes involved in lipid metabolism
the importance of LFABP in fatty acid uptake has to be considered
The aim of this study was to verify whether genetic variations in the LFABP gene may impact on plasma lipoprotein/lipid levels in the fasting state as well as on the response to a lipid-lowering therapy with fenofibrate on plasma lipids and obesity variables
We also wanted to verify whether the presence of the PPARα L162V mutation interacts with genetic variants in LFABP gene
we first determined the genomic structure of the human LFABP gene and then designed intronic primers to sequence the coding regions
and the promoter region of the gene in 24 patients showing divergent plasma lipoprotein/lipid response to fenofibrate
Sequence analysis revealed the presence of a T94A missense mutation in exon 3
Interspecies comparison revealed that threonine 94 is conserved among species
We subsequently screened another sample of 130 French Canadian subjects treated with fenofibrate for the presence of the LFABP T94A mutation
Carriers of the A94 allele were at increased risk to exhibit plasma TG levels above 2.00 mmol/l after treatment with fenofibrate [2.75 (1.03–7.34); OR 95% confidence interval (CI)]
carriers of the A94 allele were characterized by higher baseline plasma-free fatty acid levels (FFA) (p=0.01) and by a lower body mass index (BMI) (p=0.05) and waist circumference (p=0.005) than T94 homozygotes
PPARα L162V and LFABP T94A showed to have a synergistic effect on BMI (p interaction = 0.03)
These results suggest that the LFABP T94A missense mutation could influence obesity indices as well as the risk to exhibit residual hypertriglyceridmia following a lipid-lowering therapy with fenofibrate
and TG levels were enzymatically measured on a Multiparity Analyser CX7 (Beckman
This study received the approval of the Chicoutimi Hospital ethics committee
All exons and exon-intron boundaries were amplified from genomic DNA by use of specific primers derived from all 5′ and 3′ end of intronic sequences (Table 1)
The annealing temperature for all pairs was 60°C
Polymerase chain reaction (PCR) conditions were 50 ng genomic DNA
and 0.4 μmol/l primers in a 50-μl reaction
PCR products were purified (Multiscreen; Millipore
Sequencing reactions were performed using BigDye Terminator v3.0 cycle sequencing (ABI Prism
and the products were analyzed on ABI 3700 automated DNA sequencer (PE Applied Biosystems)
The gel files were processed using the ABI Prism 3700 data collection software applied biosystem version 1.1 and ABI Prism DNA sequencing analysis software (PE Applied Biosystems) then assembled and analyzed using the STADEN preGap4 and Gap4 programs
The LFABP T94A mutation does not alter any restriction site; thus
the mismatch PCR method was performed using primers LFABPex3.L-mismatch (5′-CAGTTGGAAGGTGACAATAAACTGGTGAAA-3′
mismatch is underlined) and LFABPex3.R (5′-ATACTGACCACAGGAAAGAAGTTTGGGG-3′)
Digestion products were electrophoresed through 4% agarose gel and stained with ethidium bromide
followed by digestion with Hha I restriction enzyme
and the ApoE genotype were considered in this model
odds ratios (OR) with 95% CI of reaching TG
and TC/HDL-C ratio target values associated with LFABP T94A genotype were reported following fibrate treatment
Analyses of covariance were also conducted to evaluate the mean phenotypic differences at baseline and in response to the treatment therapy between carriers and noncarriers of the LFABP T94A mutation
A 2×2 ANOVA was used to evaluate the possible interaction between LFABP T94A and PPARα L162V genotype on plasma lipid variables
Statistical analyses were performed using SAS (SAS institute
Schematic representation of the human liver fatty acid binding protein (LFABP) gene. Upper panel a representation of the human messenger RNA. The coding region is shaded, and arrows indicate translation start (met) and stop codon (UAA). The spatial localization of exons within the gene and the intron size is shown in the lower panel. The gene spans 5.1 kb of genomic DNA
Plasma triglyceride (TG) concentrations before treatment (pre-Tx) and after treatment (post-Tx) with fibrate, among LFABP T94 HMZ and carriers of liver fatty acid binding protein (LFABP) A94 allele. Data are mean ± SE. All values were adjusted for age, gender, BMI, ApoE, alcohol, and smoking
Plasma cholesterol concentrations before treatment (pre-Tx) and after treatment (post-Tx) with fibrate
among liver fatty acid binding protein (LFABP) T94 HMZ and carriers of the LFABP A94 allele
Asterisk is allowed for significant difference
No other significant difference between genotypes in reaching the target values were observed
To evaluate the interaction between LFABP T94A and PPARα L162V polymorphisms, subjects were divided into four genotype groups based on the presence or absence of the two variants. No difference was observed between the four genotype groups for waist girth, TG, FFA, LDL-C, HDL-C, TC, and fasting glycerol levels as well as for the TC/HDL-C ratio (Table 4)
carriers of both mutations tended to have a lower BMI
and the gene-gene interaction effect was found to be significant (p=0.03)
The human LFABP gene has been mapped on chromosome 2p11
we have determined the exon-intron structure of the human LFABP gene
Direct sequencing of the entire coding region of the human LFABP gene as well as exon-intron boundaries revealed the presence of an A to T substitution in exon 3
This substitution leads to a T94A missense mutation
Comparison with other species revealed that T94 is well conserved among species like Rattus Norvegicus and Mus Musculus
This suggests that the threonine 94 could be important to assure the physiological role of the protein
Effect of peroxisome proliferated activated receptor alpha (PPARα) L162V
liver fatty acid binding protein (LFABP) T94A
and their interaction on BMI (kilograms per meter squared)
sequencing of the entire coding region allowed us to identify a T94A missense mutation in the LFABP gene
Carriers of the A94 allele were at increased risk to exhibit residual hypertriglyceridemia above the therapeutic target following therapy with fenofibrate
The A94 allele is also associated with a lower BMI and waist girth and higher fasting FFA concentrations
Mutations LFABP T94A and PPARα L162V interact together to modulate BMI
Functional studies as well as longitudinal and prospective studies will be required to elucidate how the LFABP T94A mutation can lead to the observed effects
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C. Brouillette is the recipient of a studentship from the “Fonds de la recherche en santé du Québec Fonds pour la formation de chercheurs et l’aide à la recherche (FRSQ-FCAR santé)”. Y. Bossé is the recipient of a doctoral studentship from the Canadian Institutes of Health Research. M.C. Vohl is a research scholar from the FRSQ. D. Gaudet is the chairholder of the Canada research chair in preventive genetics and community genomics (http://www.chairs.gc.ca)
This study was supported by ECOGENE-21 (CIHR-CAR #43283)
Department of Social and Preventive Medicine
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DOI: https://doi.org/10.1007/s10038-004-0171-2
Journal of Assisted Reproduction and Genetics (2016)
Kadokawa Haruki Jimusho's official website for Issui Ogawa's Michibiki no Hoshi (Star of Guidance) science fiction novel series revealed on Thursday that an anime project is in the works. A "screen adaptation" project is in the works for completion in fall of 2018
The site describes the novel series' story:
and Gibraltar Kōbōsen (The Battle of Gibraltar) in 2005
Thanks to Dennis R for the news tip
[Via Yusuani]
showcases some of the best action sequences of 2021
and stunts fail to deliver a promising story
The flaw has now become a curse for an action genre where someone or the other may randomly tell you
“Action films don’t have a story
With a little bit of storytelling at its disposal
The Protege thematically visits the past of its two titular characters
Anna Dutton (Maggie Q) and Moody Dutton (Samuel L
While the Dutton’s are the best-paid assassins you may get in Protege’s universe
it is the anti-force Michael Rembrandt (Michael Keaton) who steals the show
Jackson) is an ace assassin who takes up high-profile contracts from all around the globe
Moody visits Vietnam to finish an assignment
Moody takes Anna under his wings and travels back to England
and informs him that she orchestrated the plan not for money but for Don Preda
where Anna runs an elegant bookstore at the street corner
Moody had Lucas’ location until 1998
As Anna investigates the mystery of Lucas Hayes
Anna’s techno informer Billy and Moody’s caretaker
Everything related to Lucas Hayes traces back to Anna’s homeland
Anna found out Lucas Hayes was the son of Edward Hayes
Edward was a businessman indicted for war crimes who was killed in a car explosion in Da Nang
Anna saw Moody standing in the crowd near the crime scene and speculated that Moody would have bombed Edward’s car
After his father’s murder on Christmas day
Lucas stayed in Paris until 1998 but returned to Da Nang in March 1999
He was admitted to St Quiteria Hospital on June 2nd
after which there was no record of his existence
Anna visited Edward’s business partner and Co-CEO
Vohl’s personal attorney Duquet shot Vohl without a blink and captured Anna at the company’s building
Their gang was killing anyone and everyone investigating Lucas Hayes
After a bit of an “action” struggle
Anna fled from captivity and ended up at Lucas’ last known location
The nun at the hospital showed the wrong person
only one person could give satisfactory answers to Anna’s curiosity
Anna discovered that both Moody and Edward were alive
Moody tricked Edward’s hired assassin
Moody and Anna infiltrated Edward’s stronghold on a secluded island and planned to kill him during his extravagant charity event
Edward was escorted to his “panic bunker” to save his life
Moody was waiting for him there with a ticking bomb in his bag
Edward confessed that he faked his death to protect his beloved son
Moody sarcastically laughed at Edward’s emotional plea and underlined that Edward did all to save himself
The fake death was Edward’s chance to disappear as no one looks for a dead man
Edward ran his crime syndicate from the secluded island
Moody also conveyed his addictive voyage to find Lucas
Moody felt remorseful for taking away a father from a son
How could he have known that the web of affairs of rich criminals is beyond anyone’s understanding
When the confessions were done and dealt with
The pursuit of Edward Hayes was Moody’s journey
and it didn’t hold enough closure for Anna’s character
and facing it would only bring full closure
A bleeding Anna left the island and visited the location in Da Nang
She sent the location coordinates to Rembrandt to finish the last chapter of the story
Anna had shown the disconcert to remember her haunting past
she didn’t remember it or didn’t want to remember it
and thus she didn’t want to visit Vietnam as the lands would have revived her memory
Anna remembered how Vietnamese militants killed her American father
the leader captured Anna and took her to their den
He assembled two of the one guns in front of Anna and decided to sleep with young Anna
Anna had an exceptional talent since childhood and had learned the technique of assembling guns by just observing
she pointed a gun at him and killed the three militants inside the den
It was the horrific memory Anna had been hiding all along
Rembrandt reached the militant’s den and requested Anna to drop the gun and reconcile their relationship
But Anna yearned for closure and peaceful life
She wouldn’t have been able to live it until Rembrandt’ was alive
Anna killed Rembrandt and walked out of the door
The Protege is a 2021 Action Thriller film directed by Martin Campbell